J/A+A/657/A96  Detection of the propargyl radical at lambda 3mm (Agundez+, 2022)

Detection of the propargyl radical at lambda 3 mm. Agundez M., Marcelino N., Cabezas C., Fuentetaja R., Tercero B., de Vicente P., Cernicharo J. <Astron. Astrophys. 657, A96 (2022)> =2022A&A...657A..96A 2022A&A...657A..96A (SIMBAD/NED BibCode)
ADC_Keywords: Atomic physics Keywords: astrochemistry - line: identification - molecular processes - ISM: molecules - radio lines: ISM Abstract: We report the detection of the propargyl radical (CH2CCH) in the cold dark cloud TMC-1 in the lambda 3mm wavelength band. We recently discovered this species in space toward the same source at a wavelength of lambda 8mm. In those observations, various hyperfine components of the 202-101 rotational transition, at 37.5GHz, were detected using the Yebes 40m telescope. Here, we used the IRAM 30m telescope to detect ten hyperfine components of the 505-404 rotational transition, lying at 93.6GHz. The observed frequencies differ by 0.2MHz with respect to the predictions from available laboratory data. This difference is significant for a radioastronomical search for CH2CCH in interstellar sources with narrow lines. We thus included the measured frequencies in a new spectroscopic analysis to provide accurate frequency predictions for the interstellar search for propargyl at mm wavelengths. Moreover, we recommend that future searches for CH2CCH in cold interstellar clouds are carried out at lambda 3mm, rather than at lambda 8 mm. The 505-404 transition is about five times more intense than the 202-101 transition in TMC-1, which implies that detecting the former requires about seven times less telescope time than detecting the latter. We constrain the rotational temperature of CH2CCH in TMC-1 to 9.9±1.5K, which indicates that the rotational levels of this species are thermalized at the gas kinetic temperature. The revised value of the column density of CH2CCH (including ortho and para species) is (1.0±0.2)x1014cm-2, and thus the CH2CCH/CH3CCH abundance ratio is revised from slightly below one to nearly one. This study opens the door for future detections of CH2CCH in other cold interstellar clouds, making possible to further investigate the role of this very abundant hydrocarbon radical in the synthesis of large organic molecules such as aromatic rings. Description: tableA1.dat contains the predicted transition frequencies for CH2CCH at 300K. File Summary: -------------------------------------------------------------------------------- FileName Lrecl Records Explanations -------------------------------------------------------------------------------- ReadMe 80 . This file tablea1.dat 77 4293 Predicted frequencies for CH2CCH at 300K -------------------------------------------------------------------------------- Byte-by-byte Description of file: tablea1.dat -------------------------------------------------------------------------------- Bytes Format Units Label Explanations -------------------------------------------------------------------------------- 3- 13 F11.4 MHz Freq Calculated transition frequency 16- 21 F6.4 MHz O-C Uncertainty of calculated transition frequency 23- 29 F7.4 [nm2.MHz] logInt Base 10 logarithm of the integrated intensity 31 I1 --- DOF Degrees of freedom in the partition function 33- 41 F9.4 cm-1 Elow Energy of the lower state 42- 44 I3 --- gup Upper state degeneracy 47- 51 I5 --- Tag Species tag or molecular identifier 52- 65 A14 --- QNFMT Identifies the format of the quantum numbers given in the field QN 68- 77 A10 --- QN Quantum numbers coded according to QNFMT -------------------------------------------------------------------------------- Acknowledgements: Marcelino Agundez, marcelino.agundez(at)csic.es
(End) Patricia Vannier [CDS] 10-Dec-2021
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