J/A+A/646/L1        HDCCN discovery in space and in laboratory  (Cabezas+, 2021)

Space and laboratory observation of the deuterated cyanomethyl radical HDCCN. Cabezas C., Endo Y., Roueff E., Marcelino N., Agundez M., Tercero B., Cernicharo J. <Astron. Astrophys. 646, L1 (2021)> =2021A&A...646L...1C 2021A&A...646L...1C (SIMBAD/NED BibCode)
ADC_Keywords: Molecular clouds ; Interstellar medium ; Atomic physics Keywords: astrochemistry - ISM: molecules - ISM: individual objects: TMC-1 - line: identification - molecular data Abstract: Observations of TMC-1 with the Yebes 40m radio telescope in the 31.0-50.3GHz range allowed the detection of a group of unidentified lines, showing a complex line pattern indicative of an open-shell species. The observed frequencies of these lines and the similarity of the spectral pattern with that of the 202-101 rotational transition of H2CCN point to that the lines arise from the deuterated cyanomethyl radical, HDCCN. Using Fourier transform microwave spectroscopy experiments combined with electric discharges we have succeeded in producing the radical HDCCN in the laboratory and observed its 101-000 and 202-101 rotational transitions. From our observations and assuming a rotational temperature of 5K, we derive an abundance ratio H2CCN/HDCCN=20. The high abundance of the deuterated form of H2CCN is well accounted for by a standard gas-phase model where deuteration is driven by deuteron transfer from the H2D+ molecular ion. Description: The table contains rotational transitions for HDCCN up to 300GHz. Objects: ---------------------------------------------------------- RA (ICRS) DE Designation(s) ---------------------------------------------------------- 04 41 45.9 +25 41 27 TMC-1 = HCL 2 ---------------------------------------------------------- File Summary: -------------------------------------------------------------------------------- FileName Lrecl Records Explanations -------------------------------------------------------------------------------- ReadMe 80 . This file table.dat 77 27032 Predicted frequencies for HDCCN -------------------------------------------------------------------------------- Byte-by-byte Description of file: table.dat -------------------------------------------------------------------------------- Bytes Format Units Label Explanations -------------------------------------------------------------------------------- 1- 11 F11.4 MHz Freq Frequency 12- 19 F8.4 MHz Unc Uncertainty on frequency 22- 28 F7.4 nm2.MHz Int Intensity 30- 37 F8.4 cm-1 Elow Lower state energy 40- 41 I2 --- N' Quantum number N for upper level 44- 45 I2 --- Ka' Quantum number Ka for upper level 48- 49 I2 --- Kc' Quantum number Kc for upper level 52- 53 I2 --- TSP' TSP aggregate spin number for upper level 56- 57 I2 --- F' Quantum number F for lower level 60- 61 I2 --- N" Quantum number N for lower level 64- 65 I2 --- Ka" Quantum number Ka for lower level 68- 69 I2 --- Kc" Quantum number Kc for lower level 72- 73 I2 --- TSP" TSP aggregate spin number for lower level 76- 77 I2 --- F" Quantum number F for lower level -------------------------------------------------------------------------------- Acknowledgements: Carlos Cabezas, carlos.cabezas(at)csic.es
(End) Patricia Vannier [CDS] 12-Jan-2021
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